Step 1: Concept
Simplify the algebraic expression using exponent rules.
Step 2: Analysis
The denominator $(\frac{a}{3})^{-\frac{1}{3}} + 3a^{\frac{2}{3}}$ can be rewritten as $3^{\frac{1}{3}}a^{-\frac{1}{3}} + 3a^{\frac{2}{3}}$.
Multiply both numerator and denominator by $a^{\frac{1}{3}}$ to clear negative exponents.
Numerator: $2^{\frac{1}{3}}a^{\frac{1}{3}} + 27a^{2} = (2a)^{\frac{1}{3}} + (3a^{\frac{2}{3}})^{3}$.
This follows the form $x^3 + y^3 = (x+y)(x^2 - xy + y^2)$.
Step 3: Calculation
By comparing both sides after simplification, the term $-ka^{\frac{1}{3}}$ corresponds to $-3\sqrt[3]{2} \cdot \sqrt[3]{27} a^{\frac{1}{3}}$, leading to $k = 3\sqrt{6}$.
Step 4: Conclusion
Hence, $k = 3\sqrt{6}$.
Final Answer: (D)